By Ted Mann, Emily Glazer and Dana Mattioli 

Wells Fargo & Co. is in talks to buy all or part of General Electric Co.'s biggest lending operation, a move that could help the San Francisco bank extend its lead in helping to finance midsize businesses.

General Electric is selling the portfolio consisting of $74 billion of loans to U.S. businesses as part of its plans to dismantle what was one of the U.S.'s largest banks, people familiar with the matter said.

GE is in talks with Wells Fargo as well as other bidders, the people said. Further details, including a possible price, weren't available.

It is extremely rare for such a large portfolio of loans to hit the market. Buying such a big block could be particularly attractive now because interest rates are so low, making it harder for banks to make money. For example, Wells Fargo's net interest margin, a measure of how much money it can make from lending out customer deposits, has dropped consecutively for the past 11 quarters. Last week, the bank said that margin shrank to 2.95% in the first quarter from 3.2% in the same period a year earlier.

Midsize lending is also in Wells Fargo's wheelhouse. It is one of the largest lenders to such businesses--typically companies with revenue ranging from $25 million to $500 million--and has been seeking to bolster lending in this area. The bank last year estimated it lends to about 25% of these companies, with more than $80 billion in loans to such companies in 2013, the latest data available, up from $74.2 billion in 2012.

GE considers the business up for sale to be one of the strongest parts of its GE Capital operations, providing financing for companies such as fast-food franchisees, recreational-vehicle dealerships and supermarket chains. It has more than 260,000 customers and dealers, according to GE.

Wells Fargo has already had preliminary talks with regulators about the possible acquisition. The bank is likely to continue keeping regulators, such as the Federal Reserve and the Office of the Comptroller of the Currency, abreast of its plans even if just informing them of considerations among the parties.

Any deal could be Wells Fargo's largest since its roughly $15 billion acquisition of Wachovia Corp. during the financial crisis.

If it were sizable enough, such a purchase could change the way regulators view Wells Fargo compared with its bigger competitors. Rivals such as such as J.P. Morgan Chase & Co. and Citigroup Inc. are required to set aside more capital than Wells Fargo to guard against recessions or deep losses, which would depress profitability. Wells Fargo currently is required to hold less capital as a simpler bank, but a deal like this could boost it to a higher level.

The bank is already buying part of GE's $26.5 billion portfolio of investment in office building and other commercial property. But Chief Financial Officer John Shrewsberry dropped a hint last week that more could be in the pipeline. "There is opportunity there," he said on an earnings call. "We will definitely be working closely together."

General Electric has said it would sell off $200 billion in assets over the next two years. Any agreement would signal to Wall Street that GE's exit from banking will happen even more quickly than the company has forecast. The company has publicly given itself two years to complete the process.

The move is part of a strategic shift by Chief Executive Jeff Immelt to address long-standing investor dissatisfaction with the level of credit risk at the 123-year-old company and to return GE to its industrial roots making jet engines, power turbines and MRI machines.

GE also has contacted potential buyers for its $16 billion private-equity lending business, according to some of the people.

Mr. Immelt and his management team decided in February to push forward with a plan to exit from GE Capital, according to people familiar with the matter. The executives told investors that they were driven primarily by timing: The market for financial assets is strong, and it was the right time to try to sell GE's financial operations and refocus on its industrial operations, which are expected to produce 90% of the company's profits by 2018.

GE Capital CEO Keith Sherin is leading the process to sell GE Capital's remaining businesses, amounting to about $165 billion in assets. In addition to the U.S. middle-market lending business and its private-equity lending operation, GE Capital also is trying to sell a $31 billion international commercial-lending business, a $9 billion vehicle fleet-management unit and an international consumer-banking unit that holds $37 billion in assets.

Write to Ted Mann at ted.mann@wsj.com, Emily Glazer at emily.glazer@wsj.com and Dana Mattioli at dana.mattioli@wsj.com

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